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Beilstein J. Org. Chem. 2017, 13, 762–767, doi:10.3762/bjoc.13.75
Graphical Abstract
Scheme 1: Desymmetrization of cyclohexadienone by tethered nucleophile.
Scheme 2: Scope of the transformation.
Figure 1: Chiral iminophosphorane catalysts surveyed.
Scheme 3: Convex facial additions.
Scheme 4: Attempted oxidative deacylation.
Scheme 5: Attempted desulfurization with Raney nickel.